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Saturday, May 10, 2025

Proppants for Hydraulic Fracturing in Oil & Gas and Enhanced Geothermal Wells: Frac Sand, Exxon’s New Lightweight Petroleum Coke Proppants, Ceramic Proppants, and Resin-Coated Proppants


Frac Sand Characteristics and Requirements

     Frac sand is the predominant proppant used in oil & gas wells. The American Petroleum Institute sets standards for frac sand. It has to be >99% sand or quartz. It should be in one of four “mesh” sizes. Sphericity and roundness should be at least 0.6. This is to increase permeability to fluids. It needs to have a crush resistance of 4000 to 6000 psi. A single shale well can use as much as 10,000 tons of frac sand (from 2014 data). Frac sand grain sizes range from 0.1 mm to over 2 mm. The most common range is 0.4 mm to 0.8 mm. In the U.S., most frac sand, about 75% (from 2014 data), is mined in the state of Wisconsin.

 

Ceramic Proppants

     Ceramic proppants have a higher crush strength than conventional frac sand. They can be used effectively in deeper, hotter, and higher-pressure wells, including enhanced geothermal wells. They are also easier to conduct into the fractures than frac sand. Crush strength for ceramic proppants is up to 10,000 psi. Uniformity in size, shape, and sphericity allows ceramic proppants to be conducted into the induced fractures better than less uniform frac sand. Ceramic proppants are also more stable and less likely to react chemically or thermally than frac sand. The reactions can lead to deposits on the sand, which occlude porosity over time through a process known as diagenesis. However, ceramic proppants are more expensive than frac sand and resin-coated frac sand.

     Ceramic proppants are available in three density grades: lightweight low density, intermediate density, and high density. Most ceramic proppants are made from bauxite, kaolin (aka China Clay), or a blend of both materials. Magnesium silicate and fly ash may also be used. Various additives may also be included. The alumina content of ceramic proppant correlates with pellet strength and density.

     Manufacturing ceramic proppants requires five steps: crushing, pelletizing, drying, sintering, and cooling. Sintering at 2700-2900 degrees F gives the proppants the hardness and crush strength needed.

 

Resin-Coated Proppants

     Any proppant, including sand, ceramics, and petcoke-based proppants may be coated with resin. Resin coating gives better crush strength and increased conductivity into the fractures. It also results in less flowback of crushed fines, which lower the amount of proppant that stays in place to keep the induced fractures propped open. Flowback fines can also cause problems with pumps and surface equipment. Reducing flowback fines is the key goal and function of resin-coated proppants.

     The most commonly used resins for coating are epoxy resins, furan, polyesters, vinyl esters, and polyurethane. Epoxy resins are the most commonly used for proppants due to their strength and chemical stability.

     A 2021 paper in Petroleum Science found that a certain epoxy resin-coated (ERC) proppant performed particularly well against other proppants.

Compared with uncoated ceramic proppants, the epoxy resin-coated (ERC) proppant has a high self-suspension ability, nearly 16 times that of the uncoated proppants. Besides, the hydrophobic property and the liquid conductivity of the ERC proppant increased by 83.8% and 16.71%, respectively, compared with the uncoated proppants. In summary, this novel ERC proppant provides new insights into the design of functional proppants, which are expected to be applied to oil and gas production.

 










Lightweight Proppants

     Lightweight proppants decrease the amount of energy required for proppant transport. This is very important when proppant transport is hindered by low permeability and friction losses in the ultra-long laterals, which are becoming more common in the oil and gas industry.

     One metric that distinguishes lightweight proppants from other proppants is settling speed, as shown below from a 2021 comprehensive analysis of ultra-lightweight proppants published in Petroleum. The table shows different types of lightweight proppants. These include petroleum coke proppants, hollow ceramic beads, amended walnut hulls, and many others.








     Below are the advantages of ultra-light-weight (ULW) proppants from the 2021 paper:

    






Petroleum Coke-Based Proppants

     I didn’t get to read Hart Energy’s articles about Exxon’s use of petcoke proppants, but I did find an AI-generated analysis of them, which I reproduce below.

Petroleum coke (petcoke) is a carbon-rich byproduct of oil refining, and it’s being used as a proppant in hydraulic fracturing (fracking) operations. Petcoke’s low density and potential for increased fracture conductivity are making it an attractive alternative to traditional sand proppants, especially in areas where sand is difficult to transport or when a lighter proppant is needed to reach the ends of long laterals.”

“Advantages of Petcoke as a Proppant:

Low Density: Petcoke has a lower density than sand, which means it can be suspended and transported farther into fractures using lower-viscosity fracturing fluids.”

Potential for Increased Conductivity: The structure of petcoke, with its roughness and uneven surface, can help support the fracture walls at multiple points, reducing embedment and potentially leading to higher fracture conductivity and prolonged gas flow.

Cost-Effectiveness: ExxonMobil is manufacturing its own petcoke proppant in its refineries, which helps to lower the cost compared to other proppants.”

Increased Recovery: Early results from Exxon’s pilot program using petcoke show a 15% increase in estimated ultimate recovery (EUR) in some wells.”

Considerations:

“Shape and Roundness: Petcoke grains tend to have a lower sphericity and roundness compared to sand or ceramic proppants, which can affect their packing density and behavior in the fracture.”

Ash Content: The ash content of petcoke can vary depending on the type and source.”

Strength: While petcoke can be strong enough to prop fractures, it’s important to consider its strength characteristics in different conditions.”

Environmental Concerns: Petcoke can contain sulfur and other contaminants, which need to be considered during handling, storage, and disposal.”

 

Blast Furnace Coke Proppants for Coal Bed Methane Frac Jobs

     A pair of papers, one from January 2023 and one from December 2024, address the value of coke proppants for coal bed methane wells. The problem to be overcome is known as embedment, where the proppant grains damage fracture walls, leading to blocked fractures. It is common in soft-rock formations such as coal. 







     The 2023 paper tested different types of coke as proppants. It was found that the coke made from coal in blast furnaces provided the best ultra-lightweight proppant for decreasing the embedment phenomenon. The 2024 paper reiterated that modified blast furnace coke is the most effective proppant for reducing embedment, with other advantages listed below, followed by the highlights and abstract to the 2024 paper.

“First, the coke roughness supports the fracture wall at multiple points and reduces the embedment effect, which ensures prolonged proppant conductivity within the fracture network, facilitating sustained gas flow and maximizing production rates. Additionally, the low density of coke-based proppants enables their suspension in low-viscosity fracturing fluids, thereby reducing pumping pressures, minimizing water consumption, and improving well cleaning efficiency.”

 




Proppants for Enhanced Geothermal Wells

     Proppants are a key concern for developing successful enhanced geothermal (EGS) wells, especially where reservoir temperatures are high. Hotter rocks have lower permeability, so there is a need to increase permeability to increase flow rates. Early EGS wells did not use proppant, and as a result, the flow rates were not sufficient. There are ongoing arguments about whether proppant is needed in hot rocks, as some think pumping water below closure pressures allows for “self-propping” and others think that pumping at higher pressures can lead to “hydro-propping,” but recent tests indicate that the use of proppant will be needed. Fervo Energy’s Project Red in Nevada was hydraulically fractured in 2023. The well pair achieved the highest circulation rate ever recorded in an EGS project, despite starting with a very tight initial permeability using a shale-style multistage plug and perf fracturing treatment, with conventional proppant. Those wells are now producing into the power grid. Fervo’s FORGE project tried some fracs near larger faults without proppant, and they failed to get the flow rates needed. The propped wells perform much better. However, there are some potential concerns with proppant in geothermal wells. One is that surface infrastructure cannot tolerate any sand or proppant returning to the surface. There is also concern with minerals in the proppants speeding up reactions with mineral-rich water, which can lead to plugging porosity.

     A February 2025 paper presented at the 50th Workshop Proceedings on Geothermal Reservoir Engineering at Stanford University, compared different proppants under room temperature conditions and under simulated geothermal conditions of high temperatures (300 °C) for up to 30 days. 









     The results suggest that a mixture of proppants could offer the best results. They also note that the low cost of petcoke proppants can be advantageous. The abstract and conclusion of the paper are given below:

 

ABSTRACT 

Recent advancements in hydraulic fracturing technology have significantly improved the extraction of hydrocarbons and geothermal energy from unconventional reservoirs. This study evaluates the performance of various proppant materials, including petroleum coke based proppants (PC), high-transported ultra-low-density ceramic proppants (LDC), and resin-coated ceramic proppants (RC), focusing on their crush resistance and packing strength under geothermal conditions. Utilizing the Standard procedure from API ISO 13503-2, we assessed both wet and dry proppants across two mesh sizes (10/35 and 35/60) and subjected wet samples to high temperatures (300 °C) for up to 30 days to simulate geothermal conditions.”

The room temperature test results reveal that petroleum coke-based proppants, while cost-effective, exhibit lower strength compared to ceramic proppants. Whereas the resin-coated ceramic exhibited very high stress tolerance. Notably, the crush resistance and packing strength of proppants decreased with increasing temperature, with variations observed based on proppant type and size. Specifically, petroleum coke-based proppants did not show a significant decrease in strength after exposure to high temperatures. Conversely, ceramic-based proppants experienced a noticeable reduction in strength under the same conditions. In mixed proppant tests, blending PC with LDC or RC at various ratios showed a significant reduction in fines generation and improved mechanical performance, particularly at a closure pressure of 5000 psi, which is representative of geothermal reservoir conditions. These findings provide valuable insights into optimizing proppant selection and mixing for enhanced performance in both unconventional reservoirs and geothermal applications. The study highlights the importance of tailored proppant strategies to balance cost, strength, and efficiency, contributing to the development of more effective and economical fracturing solutions.

CONCLUSION

“This study provides a comprehensive evaluation of the mechanical properties of various proppants under simulated downhole conditions. The findings demonstrate that while PC proppants are economically advantageous, they exhibit lower strength compared to ceramic-based alternatives. Among the ceramic proppants, RC proppants showed superior stress tolerance.”

“Temperature has a significant impact on proppant performance. The crush resistance and packing strength of all proppants decreased with rising temperatures; however, the extent of degradation was notably different between proppant types. PC proppants retained their strength even after exposure to high temperatures, whereas ceramic-based proppants experienced a substantial reduction in strength. The results underscore the importance of selecting appropriate proppants based on both economic considerations and performance requirements. For applications involving high temperatures, such as in geothermal systems, PC proppants might offer a more stable and cost-effective solution compared to ceramic proppants, which show more significant strength reduction under similar conditions. Further research and field testing are recommended to optimize proppant selection and mixing strategies for enhanced efficiency and cost-effectiveness in various fracturing scenarios.”

“The SEM-EDX analysis of the proppants before and after heat exposure displayed noticeable changes in the surface structure. Microcracks were more prevalent in the proppant exposed to heat, and the presence of gas release pores was observed, suggesting potential alterations in the proppant's properties due to high-temperature conditions. The findings will contribute to the selection and optimization of proppant materials for efficient and sustainable development of unconventional oil and gas reservoirs, as well as geothermal fields.”

     Another study presented at the same conference in 2023 showed that coated proppants under simulated geothermal conditions of 320 degrees C produced more fines than non-coated proppants. Results are summarized below.

The results show that the heated proppant in EGS conditions has a lower approximate packing strength and yields a higher fines percentage, indicating reduced conductivity after its exposure to high temperature fluid for 14 days. The capability of polymer coating, encapsulating and trapping fines within polymer coating, is reduced by coating degradation in high temperatures fluid, resulting in significant increase in fines percentage compared to non-coated proppants.”

 

Proppant Load as a Metric: Proppant Used Per Frac Stage Correlates with Higher Fracture Conductivity and Higher Well Production

     Along with pumping rates, the amount of proppant loaded into each frac stage provides an important method that correlates very well with better well production, indicating better fracture connectivity. As frac jobs got bigger with higher pumping rates and higher proppant loads, production rates climbed. Getting the most proppant emplaced to keep the fractures open is the goal of hydraulic fracturing, and work is ongoing to optimize the process.

 

 

References:

 

The Critical Role of Proppant in Enhanced Geothermal Systems. Mark McClure, Rohan Irvin, and John McGrath. Petroleum Connection. March 27, 2024. The Critical Role of Proppant in Enhanced Geothermal Systems – Petroleum Connection

Selection and Testing of Proppants for EGS. Sunghyun Ko, Ahmad Ghassemi, and Matt Uddenberg. PROCEEDINGS, 48th Workshop on Geothermal Reservoir Engineering. Stanford University, Stanford, California, February 6-8, 2023. SGP-TR-224. Selection and Testing of Proppants for EGS

When Fracturing for Geothermal, Is Proppant Really Necessary? Stephen Rassenfross. Journal of Petroleum Technology. March 16, 2023. When Fracturing for Geothermal, Is Proppant Really Necessary?

Exxon’s Custom, Lightweight Proppant Boosts Permian EURs by 15%. Chris Matthews. Hart Energy. December 16, 2024. Exxon’s Custom, Lightweight Proppant Boosts Permian EURs by 15% | Hart Energy

Crush Resistance and Packing Strength of Candidate Proppant for Enhanced Geothermal Systems. Sree Sujon Sutradhor and Ahmad Ghassemi. PROCEEDINGS, 50th Workshop on Geothermal Reservoir Engineering. Stanford University, Stanford, California, February 10-12, 2025. SGP-TR-229. Crush Resistance and Packing Strength of Candidate Proppant for Enhanced Geothermal Systems

Resin-coated petroleum coke as proppant particulate material and methods related thereto. Patent. Canada. CA3173741A1 - Resin-coated petroleum coke as proppant particulate material and methods related thereto - Google Patents

Assessment of the Suitability of Coke Material for Proppants in the Hydraulic Fracturing of Coals. Tomasz Suponik, Krzysztof Labus, and Rafał Morga. Materials 2023, 16(11),4083. Assessment of the Suitability of Coke Material for Proppants in the Hydraulic Fracturing of Coals

Coke-based proppant for coalbed methane technology. Rafał Morga, Krzysztof Labus, and Tomasz Suponik. International Journal of Coal Geology. Volume 295, 4 December 2024, 104647. Coke-based proppant for coalbed methane technology - ScienceDirect

Ceramic Proppants: A Specialized Alternative to Frac Sand. Carrie Carlson and Alex Ebben. Feeco International. Ceramic Proppants: A Specialized Alternative to Frac Sand

A comprehensive review on proppant technologies. Feng Liang, Mohammed Sayed, Ghaithan A. Al-Muntasheri, Frank F. Chang, and Leiming Li. Petroleum. Volume 2, Issue 1, March 2016, Pages 26-39. A comprehensive review on proppant technologies - ScienceDirect

A comprehensive review of ultralow-weight proppant technology. Review. Yong-Cun Feng, Cheng-Yun Ma, Jin-Gen Deng, Xiao-Rong Li, Ming-Ming Chu, Cheng Hui & Yu-Yang Luo. Petroleum Science. Volume 18, pages 807–826, February 21, 2021. A comprehensive review of ultralow-weight proppant technology | Petroleum Science

Hydrophobic epoxy resin coated proppants with ultra-high self-suspension ability and enhanced liquid conductivity.Fan Fan, Feng-Xia Li, Shou-Ceng Tian, Mao Sheng, Waleed Khan, Ai-Ping Shi, Yang Zhou, and Quan Xu. Petroleum Science. Volume 18, Issue 6, 15 December 2021, Pages 1753-1759. Hydrophobic epoxy resin coated proppants with ultra-high self-suspension ability and enhanced liquid conductivity - ScienceDirect

Resin Coated Proppants. Ammat Technology Company. Resin Coated Proppants | AMMAT Technology | United States

Frac Sand Mining. Alyssa Schmid. June 19, 2014. PPT - Frac Sand Mining PowerPoint Presentation, free download - ID:1986801

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