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Tuesday, September 17, 2024

Water Treatment and Purification Technologies: And Emerging Methods and Research

 

     Water purification refers to the removal of undesirable chemicals, biological contaminants, suspended solids, and gases from water. It is typically purified for drinking water but may be purified to different standards for medical, pharmacological, chemical, and industrial purposes. Water may be filtered, and stilled for sedimentation to reduce suspended solids, flocculated, chlorinated, and/or run through ultraviolet (UV) light to purify it. Confirmation of water quality is determined by chemical and microbiological testing, which, unfortunately, is relatively costly.

     Water treatment plants typically pre-treat the water through pumping and containment, screening out any large debris (not needed for most groundwater), storage for biological purification, and running through slow sand filters. Pre-chlorination to kill off any bacterial fouling of the incoming pipes has largely been discontinued as a pretreatment method due to the harmful byproducts of chlorination. It is still used sometimes to remove algae. Slow sand filters capture some contaminants and allow for biological treatment as the water runs through them very slowly. In alluvial groundwater aquifers that occur in subsurface unconsolidated river sands (alluvium), the natural flow of the water through the sand acts as a slow sand filter for the river water. Those aquifers are considered to be younger groundwater since the water filtered down through the alluvium from the river over a few years or decades. Slow sand filters are also used to treat water in swimming pools where the water is continuously filtered slowly through a large drum filled with sand. These must be replaced every so often as the pressure changes due to solids buildup.






     Aeration is often used to treat water. Packed Tower Aeration utilizes tall towers and can remove VOCs, disinfection byproducts, CO2, H2S, and other organic compounds. Multi-stage bubble aeration can remove the same compounds but is less efficient than packed tower aeration. However, it may be cheaper and more applicable to smaller water systems.  

     pH adjustment is an important water treatment technology. If the source water is too acidic then lime, soda ash, or sodium hydroxide (caustic soda) may be added to raise the pH to neutral (7). The addition of lime will increase the calcium ion concentration and the water’s hardness. Removal of dissolved gases with degasifiers is another method of raising water pH. Making the water slightly alkaline aids the coagulation and flocculation process. It also limits the leaching of lead from pipes and solders as occurs with more acidic water sources.

     Corrosion control via phosphate feeds is another water treatment step in some systems that are deemed in need of it. Phosphoric acid, zinc orthophosphate, or other compounds may be added to treat the water. These compounds can remove orthophosphates that are “believed to combine with lead and copper in plumbing materials to form insoluble compounds, thus reducing lead and copper release at the tap.”

     Coagulation and flocculation are the next steps in water treatment. Coagulation involves the addition of coagulants such as aluminum sulfate (alum) or iron III salts such as iron III chloride. Through physical and chemical processes this causes precipitation and then merging with suspended solids particles in the water which can be flocculated out. Suspended solids in water may include inorganic clay and silt particles, algae, bacteria, viruses, protozoa, and natural organic matter. Coagulation and flocculation are considered to be two parts of the same overall process. In the 1960s polymers were developed to aid flocculation and in some cases to replace the inorganic metal salt coagulants. Polydiallyldimethylammonium chloride (polyDADMAC) is a commonly used polymer to aid flocculation.

     Sedimentation in a sediment basin is the next step after flocculation. Here the water clarifies as the floc settles to the bottom of the basin. The upper part of the water is the clearest and is passed on over a weir. Overflow rates from sedimentation tanks are typically 0.5 to 1.0 gallons per minute per square foot. The tanks must be dep enough so that the water movement does not disturb the floc, or sludge that falls to the bottom. This sludge, which typically makes up 3 to 5 % of the total water volume must be periodically removed and treated. Typical detention times are 1.5 to 4 hours and typical sedimentation tank depths are 10 to 15 feet. Sludge treatment and disposal can get expensive for water treatment plants. Other clarification methods are Lamella clarifiers which involve inclined plates and tubes to increase the surface area so more particles can be removed, and floc blanket clarifiers which remove sediment by trapping it in a layer of suspended floc as the water is forced upward.  

     Dissolved air flotation utilizes pressurized air that makes bubbles when it returns to atmospheric pressure and those bubbles trap suspended solids. It is used where normal sedimentation in tanks is considered to be inadequate. In this method, the floc floats on the surface and is skimmed off while the clarified water below is transferred to the next step in the treatment process which is filtration.

     Filtration can involve the use of one or more of several types of water filters. Filtration can capture many of the pathogens, providing some disinfection, but some still get through the filters. The most common type of filter is a rapid sand filter. These have vertical layers of sand and an activated carbon layer at the top to filter out organic compounds that affect taste and odor. The filter is periodically cleaned by reversing the flow or backflushing. Compressed air may be used as well. Pressure filters are employed by some water companies where the filter medium is enclosed in a steel casing under pressure.

Advantages {of pressure filters}

·        Filters out much smaller particles than paper and sand filters can.

·        Filters out virtually all particles larger than their specified pore sizes.

·        They are quite thin and so liquids flow through them fairly rapidly.

·        They are reasonably strong and so can withstand pressure differences across them of typically 2–5 atmospheres.

·        They can be cleaned (back flushed) and reused

 




Cutaway View of a Rapid Sand Filter




     Slow sand filters require space and land as water moves slowly through them. They rely on biological treatment more than physical filtration. They utilize graded layers of sand with the finest at the top. Wikipedia via a 2014 article in Water Supply describes more interesting things about slow sand filters:

Filtration depends on the development of a thin biological layer, called the zoogleal layer or Schmutzdecke, on the surface of the filter. An effective slow sand filter may remain in service for many weeks or even months, if the pretreatment is well designed, and produces water with a very low available nutrient level which physical methods of treatment rarely achieve. Very low nutrient levels allow water to be safely sent through distribution systems with very low disinfectant levels, thereby reducing consumer irritation over offensive levels of chlorine and chlorine by-products. Slow sand filters are not backwashed; they are maintained by having the top layer of sand scraped off when the flow is eventually obstructed by biological growth.





Slow Sand Filtration



     Bank filtration involves using the sediments in a riverbank as a kind of sand filter or alluvium as shown below.







    

     Microfiltration such as ultrafiltration membrane filtration, or the chemical method of ion exchange can remove dissolved ions. Activated carbon filters can remove organic chemicals and chlorine. Nanofiltration (NF) uses semi-permeable membranes to separate and purify water by removing particles and solutes with a molecular weight between 200 and 1,000 daltons. Nanoscale graphene-based filters can remove just about anything while letting the water molecules pass through. Water softeners typically employ ion exchange to remove calcium and magnesium ions, replacing them with sodium and potassium ions. This is cation exchange since the elements are positively charged ions. Anion exchange utilizes negatively charged ions (anions). It can remove arsenic, chromium-6, cyanide, nitrate, perchlorate, per- and polyfluoroalkyl substances (PFAS), sulfate, and uranium. Deionization via ion exchange is sometimes employed following reverse osmosis with the product being high-purity deionized water. Ion exchange can also remove nitrates, arsenic, and heavy metals. Granular activated carbon filters are made from coal, peat, wood, or coconut shells. These filters can remove inorganic contaminants including antimony, arsenic, beryllium, fluoride, selenium, thallium, and uranium. They can also remove organic compounds, including those that affect taste and odor as well as disinfection byproducts and VOCs. Contaminants are trapped by adsorption

     Disinfection is the next step which kills off any remaining pathogens. Possible pathogens include viruses, bacteria, including Salmonella, Cholera, Campylobacter, and Shigella, and protozoa, including Giardia lamblia and other cryptosporidia. Disinfection is often done in a disinfection tank where the water is held to achieve sufficient ‘contact time’ with the disinfectant at the desired concentration. Chlorine compounds are commonly used for disinfection. These may include chloramine, chlorine dioxide, sodium hypochlorite (bleach), or calcium hypochlorite. Unfortunately, chlorine compounds yield potentially harmful byproducts. These include trihalomethanes (THMs) and haloacetic acids (HAAs). Both are carcinogenic in large quantities and are regulated by the EPA. Chlorine dioxide can detonate. It is fast-acting but yields chlorite as a byproduct that is regulated to low levels. Chloramines are being used more often since they don’t make THMs and HAAs, but they are less potent than sodium hypochlorite. Chloramines derive from ammonia and chlorine. They can also experience nitrification with the end results being undesirable nitrates. They can also leach metals, including lead. Chlorine compounds have limited effectiveness against pathogenic protozoa that form cysts in water such as Giardia lamblia and Cryptosporidium.





     Ultraviolet light (UV) is most effective at inactivating cysts, in low turbidity water. It is less effective in water with turbidity. It can work well in concert with chloramines. UV light can be used in conjunction with hydrogen peroxide and/or chlorine which create radicals such as hydroxyls that can oxidize contaminants. It can remove dangerous microcontaminants such as 1,4-dioxane, N-nitrosodimethylamine (NDMA), and methyl tert-butyl ether (MTBE).

     Solar UV radiation is also used in water disinfection. Ionizing radiation, bromine, and iodine are minor methods of disinfection. Fluoride is often added to water at very low concentrations to reduce tooth decay. Small amounts of phosphate ions may be added to raise pH in order to prevent the leaching of lead from pipes, which is known as plumbosolvency. In a few groundwater sources radium is removed via ion exchange. Sometimes natural fluoride levels in water are too high and it is removed via activated alumina and bone char filtering.

     Boiling water removes some pathogens. Adsorption with granular activated carbon removes many organic compounds and their tastes and odors. Home water filters and fish tanks utilize activated carbon. Metallic silver nanoparticles may also be used. They are anti-bacterial and can remove pesticide residues. Filtered water from these filters should be used quickly and the filters should be replaced regularly.

     Biological treatment of drinking water uses indigenous bacteria to remove contaminants. According to the EPA:

 

The process has a vessel or basin called a bioreactor that contains the bacteria in a media bed. As contaminated water flows through the bed, the bacteria, in combination with an electron donor and nutrients, react with contaminants to produce biomass and other non-toxic by-products. In this way, the biological treatment chemically “reduces” the contaminant in the water.”

 

     It can remove nitrates and perchlorates. It destroys contaminants so there is no need for contaminant removal.

 

     Distillation can remove 99.9% of contaminants by recondensing the vapor from boiling water but contaminants with higher boiling points can get through.

     Reverse osmosis is a common way to get high-purity water. It is often used in conjunction with nanofiltration. According to Wikipedia via Puretec Water:

 

Reverse osmosis involves mechanical pressure applied to force water through a semi-permeable membrane. Contaminants are left on the other side of the membrane. Reverse osmosis is theoretically the most thorough method of large scale water purification available, although perfect semi-permeable membranes are difficult to create. Unless membranes are well-maintained, algae and other life forms can colonise the membranes.

 

     Reverse osmosis may be single pass, double pass, or a combo of both. It is a process that is both water-intensive and energy intensive.

 









     Other methods are used to treat contaminated water such as crystallization into hydrates with low molecular weight gases such as CO2. The water is then separated from the hydrate crystals. In situ chemical oxidation (ISCO) involves injecting oxidizers into contaminated soil or groundwater. Bioremediation utilizes microorganisms to remove contaminants such as alkanes, perchlorates, and metals. It is also used for contaminated soil and groundwater. Hydrogen peroxide (H2O2) is very good at disinfecting water. It can be delivered from chemical plants but is apparently much more potent if made onsite utilizing a gold-palladium catalyst to make the H2O2 from ambient hydrogen and oxygen. It is very good at killing E. coli bacteria.

     Distilled, or demineralized water may upset a person’s natural fluid balance. It increases the elimination of electrolytes. There are recommendations for safe, ideal, and non-safe magnesium concentrations, calcium concentrations, and water hardness. High water hardness has been linked to increases in gallstones, kidney stones, urinary stones, arthrosis, and arthropathies.

     Emerging water treatment technologies include improvements in nanotechnology, advanced oxidation processes (AOPs), electrocoagulation, forward osmosis for salt removal, membrane distillation, biological nutrient removal to remove nitrogen and phosphorus, carbon nanotube filters, solar desalination, microbial fuel cells which use particles in water to make electricity, and emerging nanomaterials.

 

 

Portable and Home Water Treatment

  

     Home water filtration systems utilizing activated charcoal are now very common. For instance, I have a Brita filter. One new trend in portable water treatment is electric water pitchers. These work well but the filters need to be replaced every 200 gallons or every three months, and the filters cost from $20 to $60. Thus, this is mainly a solution for those who can afford it.

 

 

Safe and Clean Drinking Water for People Who Need It and New Ways to Help

 

     Millions or even up to 2 billion people around the world still lack access to safe and clean drinking water. The problem is most prevalent in rural areas where people get water from rivers, lakes, or hand-dug wells. One emerging solution utilizes an aluminum foil coated with a special material called layered double hydroxide (LDH). This material acts like a magnet, attracting and trapping microbes. It was developed by an environmental engineer. It is being touted not as a standalone treatment but as a complementary one that is inexpensive and fast-acting.

 

In laboratory tests we found the LDH foil remarkably efficient, removing over 99% of E. coli bacteria, a common indicator of water contamination, from water samples within a few hours. We found that its efficacy also extends beyond E. coli, targeting a wide range of waterborne pathogens, including bacteria, viruses and parasites. This means that the LDH foil offers comprehensive protection against various diseases.”

 

     The process relies on “electrostatic attraction, drawing the microbes towards the LDH foil like iron filings to a magnet. Other chemical and physical forces contribute to making pathogens bind to the LDH surface, ensuring their effective removal from the water.”

     This solution is looking promising for use in Africa where there is a need for clean water access. The LDH foil can be provided for less than $7 per person annually. More research is needed, and field trials are underway for this emerging inexpensive clean water solution.

 

Nanoconfined Single Atom Catalysts (SACs) – New Research for Advanced Oxidation Processes Looks Promising but Still Needs Tweaked

     New research from a paper in Nature is improving the technique of advanced oxidation processes (AOPs) via nanoconfined single-atom catalysts. According to Tech Xplore:

This new method resulted in an astonishing 34.7-fold increase in the rate of pollutant degradation compared to traditional methods. The efficiency of oxidant use also improved significantly, from 61.8% to 96.6%. The system proved to be highly effective in degrading various electron-rich phenolic compounds, demonstrating robustness in different environmental conditions and maintaining high performance in real lake water tests.”

     According to the paper’s abstract:

The introduction of single-atom catalysts (SACs) into Fenton-like oxidation promises ultrafast water pollutant elimination, but the limited access to pollutants and oxidant by surface catalytic sites and the intensive oxidant consumption still severely restrict the decontamination performance. While nanoconfinement of SACs allows drastically enhanced decontamination reaction kinetics, the detailed regulatory mechanisms remain elusive.”

 

 

References:

 

Study reveals new catalytic pathway for efficient water pollution control. Science X staff. Phys.org. August 27, 2024. Study reveals new catalytic pathway for efficient water pollution control (msn.com)

Nanoconfinement steers nonradical pathway transition single atom fenton-like catalysis for improving oxidant utilization. Yan Meng, Yu-Qin Liu, Chao Wang, Yang Si, Yun-Jie Wang, Wen-Qi Xia, Tian Liu, Xu Cao, Zhi-Yan Guo, Jie-Jie Chen & Wen-Wei Li. Nature Communications volume 15, Article number: 5314 (2024), Nanoconfinement steers nonradical pathway transition in single atom fenton-like catalysis for improving oxidant utilization | Nature Communications

Water purification. Wikipedia. Water purification - Wikipedia

Water treatment. Wikipedia. Water treatment - Wikipedia

The Future of Water Purification Technology, Water Filter Direct. Blog. July 19, 2023. Revolutionary Leap: Water Purification Technologies Reshaping Our Future – Water Filter Direct

Emerging Trends in Water Purifier Technology: 2023. Drink Prime. Latest Water Purification and Filtration Technology (drinkprime.in)

Safe Drinking Water Act: Overview of Drinking Water Treatment Technologies. U.S. EPA. Overview of Drinking Water Treatment Technologies | US EPA

Aluminum foil that can clean water—researchers develop coating that attracts and traps dangerous microbes. Taufiq Ihsan. TechXplore. September 2, 2024. Aluminum foil that can clean water—researchers develop coating that attracts and traps dangerous microbes (msn.com)

Tap into technology: New innovations in water filtration systems. Yackulic Khristopher. Android Headlines. August 26, 2024. Tap into technology: New innovations in water filtration systems (msn.com)

Influence of operating parameters on the performance of a household slow sand filter. Abhilash T. Nair; M. Mansoor Ahammed; Komal Davra. Water Supply (2014) 14 (4): 643–649. Influence of operating parameters on the performance of a household slow sand filter | Water Supply | IWA Publishing (iwaponline.com)

The Basics of Reverse Osmosis. Puretec. The Basics of Reverse Osmosis | Puretec Industrial Water (puretecwater.com)

 

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