Sunday, August 20, 2023

Air Pollution and Air Quality Monitoring: Issues, Compliance, Equipment, and Trends


     In the U.S. the EPA and state environmental protection agencies design and deploy air monitoring networks based on where potential sources of air pollution can be found and prevailing weather patterns near those sources. However, these stationary installations, though the most accurate, are expensive to deploy and generally have inadequate coverage.

 

 

Clean Air is a Public Good 


     People have basic expectations that they will not have to be exposed to toxic air pollution. We know without a doubt that certain pollutants in the air cause serious health problems. Thus, monitoring air quality supports a clear public good: clean air. Air quality is one of the biggest environmental justice concerns. People who live near landfills, cement plants, industrial facilities, power plants, and many other potential sources of air pollution are rightfully concerned about air quality. Air quality is more of a concern in certain places like California due to weather inversions that increase smog, particulate matter, and NOx exposure.  

     One key study that confirmed the detrimental effects of air pollution on children was the Children’s Study, which began in Los Angeles, California in 1990. Los Angeles routinely has among the poorest air quality in the country, due in significant part to smog inversions. Researchers suspected that ground level ozone would be the culprit for decreased lung function in children. Children are great as subjects in such a study since lifestyle issues of adults like smoking do not have to be filtered out. Instead of ground-level ozone, they found that the culprit was particulate matter, mainly 2.5 PM, which can be breathed into the lungs. As air quality improved, lung function in children improved, strongly confirming the connection between air quality and lung function.

     Air pollution can affect humans and other mammals in multiple ways. Depending on the pollutant there are respiratory, cardiovascular, carcinogenic, reproductive and hormonal, and neurological effects. Air pollution also impacts ecosystems. It even affects materials including metals, stone, fabrics, paints, paper, glass, and rubber. These effects are mostly chemical effects. Quantifying and risk-assessing air pollution is a complex science. Indoor pollution is another area of concern. In particular, the dangerous substances of asbestos and radon are of great concern. Formaldehyde outgassing from particle board, VOCs, and combustion gases like CO and NOx can also be of concern.

     Unfortunately, some ‘anti-green’ advocates like lawyer and author Steve Milloy and contrarian scientist James Enstrom, have strived to dispute the very obvious findings that air pollution is dangerous. One need only look at the London Smog of 1952 when smog from burning coal was kept at ground level for four days by a weather inversion. That event is estimated to have killed 4000 people and made 100,000 people ill. Air pollution is harmful. That is indisputable. The level of harm is, of course, dependent on exposure, length and frequency of exposure, and concentration of pollutants.

 

 

Air Quality Improvements

 

     Fortunately, due to regulation, compliance with regulation, and the development of air monitoring networks, air quality has improved in the U.S. It has improved tremendously since the implementation of the Clean Air Act, which was enacted in 1970 and amended in 1990. Improvements have continued to the present time. The EPA reported in 2020:

 

Nationally, the concentration of ground-level ozone has decreased 21% from 2000 to 2019. All other air pollutants regulated under NAAQS – sulfur dioxide, lead, carbon monoxide, nitrogen dioxide and particulate matter – have also significantly decreased thanks to technological advances and various air quality management and control strategies developed and implemented at the local, state, regional, and national level.” 

 

 

Information Sources

 

     For my post here I am relying heavily on the excellent and informative blog of Air Quality Education Specialist Sienna Bishop at California-based air quality company Clarity. There is a clear need for a greater density of air quality monitoring networks around industrial sites, dense cities with significant traffic, and in other places where air quality may be a concern. There is also a need for more sensors, and more points of measurement. Newer, less expensive sensors can be deployed in more places to keep monitoring networks from missing pollution sources. Data gaps can be filled in from other sources, including satellite data. Air monitoring companies and professionals can help fill in these gaps. I am also relying on lots of information from the EPA, some from state agencies, environmental groups, air monitoring companies and professionals, and books published about air pollution, including Daniel Valero’s massive tome Fundamentals of Air Pollution.

 

    

National Ambient Air Quality Standards (NAAQS) and the Six Criteria Pollutants

 

     The National Ambient Air Quality Standards involve the six criteria pollutants: nitrogen oxides (NOx), sulfur oxides (SOx), ozone (O3), carbon monoxide (CO), lead (Pb), and atmospheric particulate matter (PM 2.5 in particular, but also PM10). These criteria pollutants have specific concentrations, beyond which they are considered to be in non-attainment. The map below from 2017 shows which counties around the country are in non-attainment and for how many of the six criteria pollutants.


 



         Source: U.S. EPA






Source: U.S. EPA



     There are many different sources of the six criteria pollutants and different reasons why some areas are more prone to be in non-attainment. Combustion of fossil fuels in power plants, industrial facilities, mining, transportation, and agriculture are major sources. In parts of California, Nevada, Arizona, Utah, Wyoming, and Colorado there are weather inversions that can keep these pollutants from dispersing and keep them near ground level for longer periods of time and at higher concentrations. Particulate matter can come from multiple sources, including smoke and dust of many types. Particulate matter smaller than 2.5 micrometers (PM 2.5) is the most dangerous type of PM since it can be readily breathed into the lungs. Along with the six criteria pollutants there are other dangerous pollutants such as volatile organic compounds (VOCs), airborne industrial chemicals, silica dust, and many others.

 

 

Natural Sources of Air Pollution


     As many in the Midwest and Northeast were reminded this summer of 2023, there are natural sources of air pollution that can be dangerous. These include volcanic eruptions, sandstorms, dust storms, pollen, and wildfire smoke. Areas prone to these events where people are exposed also have seen negative health effects. I did stay indoors as much as possible during the poor air quality days but when I did go outside for any length of time I noticed solids in my nose, somewhat like what we used to call rather crassly “sawdust boogers!”

 

 

Dangers of Wildfire Smoke and the Importance of Filtration and Monitoring

 

     Recently, my local Nissan dealer offered a free cabin air filter change due to the wildfire smoke. I took them up on the offer. I also recently learned (and relearned) that the air recirculation button in the car is essential when running the A/C on hot days because it makes the A/C cool better and run more efficiently by cooling air inside rather than bringing in hot air from outside and cooling it. This improves gas mileage and may extend the life of the A/C. It is also better at keeping out toxic air, say the nasty exhaust from someone ahead of you, or of industrial stench. The times not to use it are in the winter or at certain moisture levels when it can cause window fogging. On long drives with multiple passengers, you should periodically bring in fresh air from outside to keep CO2 levels from getting too high.

     According to the European Commission, global wildfire smoke is estimated to cause 339,000 premature deaths per year. Wildfire smoke can cause air quality concerns and alerts far away from its source as we discovered this year here in the U.S. Midwest and Northeast, far away from Canadian wildfires. What wood is being burned can also add to the harm. Burning poison ivy can cause severe irritation. I discovered this when we visited some acquaintances years ago who burned a large campfire that had significant amounts of poison ivy. My young son was strongly affected, with the poison ivy going systemic. He swelled up and was sick for a week or two and had to be treated with cortisone shots. It was a scary experience.

     Real-time air quality monitoring can help us to know local air quality. This summer, I have been relying on air quality data on my iPhone weather app, which always has a frequently updated air quality index for each location. In areas where wildfire smoke is more common and more frequent, it is important to establish air quality monitoring networks with many data points that are updated frequently. Knowledge of local air dispersion patterns and timing, often affected by terrain, is essential to expanding coverage. Local, high-resolution data, with greater coverage often provided by low-cost sensors, can be helpful in this regard. For most of us away from wildfires the Air Quality Index (AQI) is usually sufficient to keep us informed but to people in more frequent poor air quality zones, there are other air quality monitoring networks and platforms such as Air Now that can give site-specific information about AQI and pollution events like wildfire smoke concentrations.


 


Source: The Enhanced Air Sensor Guidebook. U.S. EPA. September 2022. ENHANCED AIR SENSOR GUIDEBOOK.PDF

 


Source: The Enhanced Air Sensor Guidebook. U.S. EPA. September 2022. ENHANCED AIR SENSOR GUIDEBOOK.PDF



The Construction Sector is a Major Source of Air Pollution

 

      23% of air pollution, including 30% of PM10, 8% of PM2.5, and 4% of nitrous oxide emissions can be attributed to the construction sector, according to the 2019 London Atmospheric Emissions Inventory. It is the highest sector source of PM10. The dust produced from construction and demolition is a major source of particulate matter. VOCs, NOx, SOx, CO, and PM2.5 from diesel-powered heavy equipment are other sources of pollutants.

     Construction project managers should consider air quality in their projects and plan to minimize unnecessary dust and equipment emissions. Spraying water for dust control is one option. I have seen this used quite a bit in the oil and gas industry on dusty lease roads. Mulch is another option that can be even more effective. Windbreaks can help. Some sites can benefit from setting up air monitoring stations. Dust control is especially important in arid regions. Other measures that can be helpful are proper waste management and disposal and utilization of low-emissions equipment and machinery. Electric equipment and machinery, though not widespread, can reduce emissions as well as noise pollution. Another advantage of electric construction equipment is that it can be built smaller, which makes it easier to maneuver in smaller spaces. This is important since most construction happens in urban environments. The electrification of construction equipment is moving faster and is thus far more applicable in the near term than the electrification of agricultural equipment for these reasons. Sienna Bishop notes that air quality monitoring equipment needs to be frequently maintained and calibrated to be effective. Her company, Clarity, offers a sensing-as-a-service model that can be a good choice for construction projects.

 

 

Air Pollution from Traffic in Big Cities

 

     Big cities are also dense cities, with large amounts of people, vehicles, and equipment in small spaces, relative to other areas. While the density of big cities can mitigate emissions in many ways, the effects of density on air quality are not one of those ways. Dense traffic, often slow-moving and idling, means poor local air quality. Particulate matter, nitrogen dioxide, volatile organic compounds, and ground-level ozone are the most common traffic pollutants. Emissions policies for cities such as London’s Ultra-Low Emission Zone (ULEZ) can help to improve city traffic pollution. Dense air quality monitoring coverage in vulnerable areas can measure it. The European Environment Agency reported that from 2014-2020 two-thirds of reported air quality exceedances were in areas of dense city traffic and were mainly due to nitrogen oxide (NOx) emissions. This is likely due to the high NOx emissions of diesel, which is very common in Europe, compared to the U.S. where gasoline is the dominant fuel. Diesel engines combust diesel at much higher temperatures than gasoline engines combust gasoline, resulting in up to 10 times the NOx emissions, although newer diesel engines produce much less than that. As mentioned, traffic congestion and idling are major factors in localized air quality concerns. Congestion can also lead to a buildup of precursors to ground-level ozone.

     Long-term solutions to traffic can include better urban design and more availability of public transportation. Alternative transport such as walking and biking can also help if infrastructure is available and convenient.

     Air quality monitoring is essential to understanding local traffic pollution patterns. People living in areas with frequent weather inversions are at the highest risk from traffic pollution. A newer strategy for addressing traffic pollution is Intelligent Transportation Systems (ITS). “ITS collect, analyze, and communicate data related to transportation in order to improve its efficiency, mobility, and safety and can also work to reduce impacts on the environment. ITS also equips transportation users with more information that helps them to reduce their travel time, travel more safely and comfortably, and minimize traffic problems they may encounter.” The EPA models traffic emissions with their complex MOBILE6 model, which provides exhaust and evaporative emissions calculations for a wide variety of traffic pollutants.

     Fortunately, traffic emissions are magnitudes better per vehicle than they were in the past (up to 99% better than in the 1960s and up to 90% better than in 1998) and city air is much cleaner than in the past. VOC emissions have also dropped by 99% in the past 50 years. Regulations such as the Clean Air Act have led to these improvements and vindicate the usefulness of environmental protection as a societal good.


     I attended a local blues festival a few years ago that was right on the Ohio River. There were quite a few boats quite close in the water idling their diesel engines. The air was heavy with the smell of diesel. As it was a long festival I'm guessing the particulate exposure was at unhealthy levels. I read recently that the EPA has slowed its cracking down on altering pollution control equipment on diesel engines and the trend known as "rolling coal." I still see it occasionally, but apparently, the practice is out of favor. This is good. Most of us don't want to see arrogant rednecks asserting their freedom to pollute. It's rude and inconsiderate.

 

 

Air Quality Monitoring for Mining and Industry

 

     Mining and industry, including the oil and gas industry, are major sources of air pollution. The best way to understand and monitor these sites is with continuous air quality monitoring. Factories, oil refineries, metals mines, coal mines, coke plants, and petrochemical facilities are especially major sources of criteria pollutants, VOCs, and other pollutants. It is common for continuous air quality monitors to be installed at the perimeters of these facilities.

     Air quality monitors for pollutants and dust levels are essential and required within mines. Coal dust, and more commonly these days, silica dust, are major causes of black lung disease and silicosis which often leads to debilitating illness and death. Airflow monitors, toxic gas detectors, temperature, pressure and humidity level sensors, and complete mine air quality stations (MAQS) are commonly utilized within mines. Along with particulates and dust other toxic airborne pollutants that may be present in metal and/or coal mines include arsenic, trioxide dust, asbestos, antimony, iron, lead, and nickel. Adequate ventilation, adequate filtration, adequate personal protective equipment, and continuous air quality monitoring are essential in mines.

     Anemometers that measure wind speed and direction are also essential for outdoor sites to understand the potential for air pollution build-up. Long-term and continuous monitoring are obviously the best choices for understanding weather patterns, and the potential for air pollution events.

     Mining, smelting, and ore processing methods can all contribute to air pollution. Smelting, which utilizes very high-temperature heat, can produce airborne toxins such as lead, sulfur, mercury, sulfur dioxide, zinc, cadmium, and uranium. Coal-fired power plants can also produce these toxins and more along with criteria pollutants and a build-up of heavy metals in coal ash sludge. Mitigation methods for outdoor facilities include dust suppression including sprinklers, windscreens, more frequent vehicle and equipment maintenance, and wet drilling. When I worked frequently at oil and gas wells in the early 1990s, during air drilling they sometimes drilled dry, known as dusting, which produced copious amounts of dust, which quite obviously was potentially dangerous. I did maintenance very close to where dust was coming out, often unclogging pipes clogged with dust. There was no air monitoring at the time and little effort or incentive to mitigate the dust. That probably did not meet OSHA standards then and certainly does not now. Quarries are another source of dust. I have written on this blog about historical Berea Grit quarrying in northern Ohio and the many workers who died of silicosis. I have also written about Black Lung disease and how its resurgence is really related to something called slope mining where mining machines cut through high-silica areas between coal seams which exposes miners to high levels of silica dust, the major cause of silicosis.   

     Promoting sustainable mining practices can decrease pollution and greenhouse gas emissions. This includes the electrification of some equipment and processes. Diesel-electric hybrids and other lower emissions technologies can also be utilized. According to the Canadian Mining Journal, 50% of the energy consumed by mining operations is used to run the necessary ventilation systems. They recommend the use of more energy-efficient automated ventilation systems. These systems can optimize conditions better than manual systems, thus improving safety as well as cost.

     In the oil & gas industry the use of diesel-electric hybrid drilling rigs, E-fracs, utilizing braking on drilling rigs, automated drilling rigs, drilling with natural gas power, and using gas-blending can all reduce emissions at well sites. In E-fracs it is common for companies to utilize field natural gas to run “gen sets” which can be sets of reciprocating natural gas engines or better yet natural gas turbines (similar to jet engine turbines). These act as a power plant to power up the electric pumps used for pressure pumping required for hydraulic fracturing. The emissions and pollution reductions compared to using diesel generators are enormous. Many truck trips to deliver diesel fuel are eliminated as well. Some LNG liquefaction facilities have been electrified and some are partially powered by renewables such as wind and solar. I actually wrote and self-published a book in 2022, called Natural Gas and Decarbonization, which covers many of these topics in detail. Drastically lower air pollution per drilling pad, per pipeline, per facility, is one of the results of these new technologies and processes. After initial investments, E-fracs and many of these innovations are cheaper to operate than diesel-powered ops.

 

 

Clean Air Act Compliance

 

     The EPA monitors compliance with the Clean Air Act directly or through state environmental agencies.

They do this in several program areas including 1) The Acid Rain Inspection and Trading Program – which focuses on reducing the pollutants that cause acid rain: sulfur dioxide and nitrogen oxides (NOx), from the power sector, mainly from coal-fired plants. Pollution allowances are traded according to a long-established cap-and-trade system that relies on market-based incentives; 2) Applicability Determination Index (ADI) – this is basically a database that helps operators or source owners determine whether a rule applies to them or to request monitoring that may be different from standards; 3) Asbestos Demolition and Renovation – this falls under the Asbestos National Emission Standards for Hazardous Air Pollutants (NESHAP) program and involves asbestos emissions from mining, manufacturing, demolition, renovation, and waste disposal. Applicable sites are inspected by EPA or state personnel; 4) EPA's Clean Air Act Mobile Sources Program – applies to developing and enforcing air pollution standards for engines and vehicles, big and small, and all fuels used in them; 5) National Emission Standards for Hazardous Air Pollutants (NESHAP) Air Toxics – this program area establishes standards and maximum achievable control technology (MACT) for hazardous air pollutants (HAPs); 6) New Source Review/Prevention of Significant Deterioration (NSR/PSD)- this program area deals with new sources and developing and improving standards by establishing  Best Available Control Technology (BACT) or Lowest Achievable Emission Rate (LAER) technology, both of which may be changed as newer and better technologies become available; 7) Prevention of Accidental Releases – this section is involved with identifying hazards and preventing accidental releases; 8)  Standards of Performance for New Stationary Sources – this program area develops standards known as New Source Performance Standards (NSPS): “The NSPS apply to new, modified, or reconstructed affected facilities in specific source categories such as manufacturers of glass, cement, rubber tires and wool fiberglass. As of 2012, EPA had developed 94 NSPS. EPA can delegate the responsibility to implement and enforce the NSPS (or a subset) to its partners (states, local, territorial, or tribal), however, even when delegated to the states, EPA retains authority to implement and enforce the NSPS;” 9) Stratospheric Ozone Protection including chlorofluorocarbon (CFCs) and other Ozone-Depleting Substances (ODS) – this section is involved with protecting the stratospheric ozone layer which protects Earth’s inhabitants from harmful UV rays. It has been degraded by CFCs and HFCS, refrigerants used in refrigeration and air conditioning that have been largely phased out; 10) wood heaters – these are major sources of dangerous particulate matter – much worse for humans than say, natural gas stoves. The EPA tests and certified wood stove models for compliance; 11) Stack Testing – the program area tests smokestacks to determine compliance and follows the Clean Air Act National Stack Testing Guidance; 12) The Risk Management Plan Rule (RMP Rule) – this program provides guidance for chemical accident prevention at facilities using extremely hazardous substances. The rule requires companies that use certain flammable materials and toxic chemicals to develop risk management programs that must be approved by EPA and resubmitted every five years; 14) Area Source Rule Implementation Guidance - provides guidance regarding the implementation of the CAA Area Source Rules. This involves 30 HAPs identified by EPA in developing its Urban Air Toxics Strategy for managing HAPs in urban areas.

 

 

Better Air Quality Saves and Extends Lives, Improves the Environment, and Improves the Economy

 

     It is indisputable that air pollution is harmful and that mitigating it is beneficial. Studies have also shown that the benefits of mitigation exceed the costs by a ratio of 30:1. Thus, there are obvious economic benefits to improving air quality. It avoids significant health care costs, lost work, and lost productivity. This is simply because air pollution contributes to many health problems including heart disease, stroke, asthma, cancer, low birth weight, and likely many more conditions. Thus, healthier air supports a healthier economy. Air pollution also negatively affects plants and ecosystems. It can reduce agricultural yields, especially ground-level ozone. These effects also increase air pollution’s cost to society. Nitrogen oxides and ammonia can negatively affect ecosystems and contribute to eutrophication. Sulfur dioxide, nitrogen oxides, and ammonia can contribute to the acidification of soils and bodies of water which can lead to loss of biodiversity.

 

 

Regulatory-Grade Air Quality Monitoring Equipment

 

     Governments and environmental agencies utilize high-quality air monitoring equipment with strict standards for measurement in order to support air quality policies. There are two classes of these compliance monitors: Federal Reference Methods (FRMs) and Federal Equivalent Methods (FEMs). According to the EPA: FRMs are “designed to provide the most fundamentally sound and scientifically defensible concentration measurement.” FRMs are the gold standard. FRMs are “intended to provide a comparable level of compliance decision-making quality as provided by FRM.” These equivalent methods may be cheaper and not quite as good as the standard FEMs/FRMs but can add many high-quality/high-accuracy data points to the network. FEMs and FRMs are actively reviewed in terms of new designs and upgrades. The criteria for evaluating new designs and upgrades are as follows: accuracy, precision, range, detection limit, pollutant specificity, freedom from co-pollutant interferences, noise, drift (short-term and long-term), lag/rise/fall (gas analyzers), and multi-site measurement performance. Each of these specs has strict testing and acceptance requirements. They also need to be properly sited and have competent instrument setup, calibration, operation, maintenance, and troubleshooting. They are also periodically audited according to EPA’s Performance Evaluation Program (PEP). EPA’s high-quality specs for FEMs/FRMs have led to these EPA-approved devices being sold to governmental regulatory agencies around the world.

     FEMs/FRMs are expensive, typically $15,000 to $50,000 per monitor, and can often require a temperature-controlled environment and routine calibration and maintenance by skilled technicians, which increases operating costs. These devices can be quite limited in terms of siting requirements. The high cost and siting issues mean lower coverage for a process that works better with more data points. Thus, air quality with FEMs/FRMs is more regional rather than local. There are, however, good ways to fill in the missing data gaps. One is mobile air quality monitoring, which can be FEM/FRM equipment or lower-cost sensors set up in vehicles. Mobile air quality monitoring can increase spatial resolution. It can, however, miss specific pollution events. Another method to increase data coverage is stationary low-cost sensors, discussed below.

     Calibration is very important to both FEMs/FRMs and sensors. EPA defines it as follows: “procedures for checking and adjusting a reference instrument’s settings so that the measurements produced are comparable to a certified standard value.” Frequent calibration is often recommended and required. Weather parameters such as relative humidity, wind speed, wind direction, sunlight, and cloud cover also affect data quality and must always be considered in the interpretation of data.

 



State and Local Air Quality Network Coverage (2017). Source: U.S. EPA


 

Non-Regulatory-Grade Enhanced Air Quality Sensors to Fill in Data and Pinpoint New Sources

 

     These sensors have the advantage of being low-cost so that many can be employed to significantly increase data coverage and spatiotemporal resolution. They can be deployed quickly to respond to potential new emission events. There are many types, some requiring dedicated electricity service, and others with Wi-Fi, solar-charged batteries, GPS, display screens, weather sensors, and cloud connections. Sites close to pollution sources and near vulnerable populations can be given good coverage with low-cost sensors.

     Sensors need less training to operate but may need more training to interpret. They are quite portable. They vary in quality and not enough is yet known about their lifetimes as some can be short-lived and some may lose sensitivity over time. Original Equipment Manufacture (OEM) sensors may be “raw” optical, metal oxide, or electrochemical types, so only a few types for a given pollutant. One or more OEM sensors may be integrated into a device. Particulate matter (PM) sensors use optical sensors. Particles scatter light from a laser or LED as they move through the measurement cell. The detector measures the scattered light to estimate the volume of particles or the number of particles. The count is then converted to a mass concentration based on mass calibration factors or density. High humidity can cause the mass of particles to be over-estimated. Electrochemical sensors and metal oxide sensors are used for gases such as nitrogen dioxide and ozone. Electrochemical sensors are sensitive to humidity and temperature and have low power needs. Metal oxide sensors have higher power requirements due to the need to heat up the sensor in order to increase sensitivity. There are many manufacturers of air quality sensors. Some are interpreted immediately, some on the cloud, and others after the data has been adjusted according to algorithms. According to EPA:

 

Data adjustments and algorithms take many forms:

• Factory “calibration” > Manufacturer “calibration” > Field collocation > Network

correction check

• Manufacturer applied data correction > user applied data correction

• Simple linear regression > more complicated data model > machine learning/artificial

intelligence (AI)”

 

     There are many factors that make different sensors vary and sometimes provide questionable data. One method of performance evaluation of sensors is to co-locate them with FEM/FRM equipment and compare the results. Co-location can also be used to adjust or correct sensors with data adjustment equations that result in better matches with FEMs/FRMs. Sensor drift can also be better understood with co-location. Temperature, humidity, drift over time, co-pollutants and noisy data can all interfere with sensor accuracy. Since many pollution emission events may be temporary, these issues could render the data useless or erroneous. FEMs/FRMs have much better diagnostic parameters that can be validated. Ways to validate data with sensors include co-locating with FEMs/FRMs, comparing and correcting to other sensors in a close network, and drive-by validation with mobile monitors. While sensors have lower-quality data, they can be useful when integrated with FEMs/FRMs. Since sensors are deployed in less controlled environments than FEMs/FRMs, they also need to be cleaned and maintained more as they can be more affected by things like dust and moisture.



Key Differences Between Reference Monitors and Low-Cost Sensors. Source: U.S. EPA


     An important factor for evaluating an air sensor is its response time to an emission event. A sensor with a quick response time, or high time resolution, can respond better to rapid changes in pollutant concentrations at a stationary point, as the graphic below shows:

 

 


   Source: The Enhanced Air Sensor Guidebook. U.S. EPA. September 2022. ENHANCED AIR SENSOR GUIDEBOOK.PDF

 


   In 2014, EPA first published the Air Sensor Guidebook which can support users in planning and collecting air quality measurements using air sensors. The latest version is the Enhanced Air Sensor Guidebook, last published in September 2022. It is a great resource, not only for air quality sensor information, but for air pollution studies in general. It gives useful strategies for developing sensor networks, including strategies for quality assurance (QA) and quality control (QC). EPA also provides information, including videos, on their Air Sensor Toolbox website.

 

 


Source: The Enhanced Air Sensor Guidebook. U.S. EPA. September 2022. ENHANCED AIR SENSOR GUIDEBOOK.PDF


Satellite Air Quality Monitoring

 

     Another way to increase air quality data coverage is with satellite data. One such satellite is NASA’s Moderate Resolution Imaging Spectroradiometer (MODIS). Air quality monitoring from satellites is based on how sunlight is scattered by ambient particles. The way NASA describes it is as follows: “Satellites measure backscattered radiation, from which vertical column densities can be calculated.” This is a form of remote sensing. Micro-satellites can photograph the entire surface of the Earth each day with a resolution of about 3 meters per pixel. Researchers at Duke University have used that data combined with metrics such as wind, relative humidity, temperature, and other parameters combined with meteorological data and trained the model through machine learning to predict local PM 2.5 levels. Though accuracy is much lower than other measurements the spatial resolution can be phenomenal.

     Researchers Alan Krupnick and Daniel Sullivan have found that for PM2.5 “EPA and its land-based monitoring network have failed to identify 54 counties and another 25 million people in the United States who live in areas that violate these air quality standards.” They think that the reason is simply that monitors are too sparse, and they think that satellite data is the best way to fill in the gaps. The article is from 2020 but they think that satellite data can do better than low-cost sensors for filling in the data. The authors suggest that pollution point sources and hotspots can be missed, even when abiding by EPA’s recommendations for monitor placement, due to prevailing wind patterns, distance from point sources, and other factors. Another huge problem they note is that monitors don’t run all the time, especially older ones. They found that while new PM2.5 monitors typically run more than 300 days per year, “56 percent of PM2.5 monitors gathered data on fewer than 121 days in 2015, and 23 percent gathered data on fewer than 80 days.” They also note that since EPA announces when monitors are working or not working, this gives incentives for some companies to pollute more when monitors are off-line. They think satellite data can help.

     Instead of directly measuring PM2.5, satellites measure aerosol optical depth (AOD) from which the density of aerosol particles can be estimated. The measurement involves the difference between the solar radiation at the top of the atmosphere and the radiation that reaches the Earth’s surface. When more airborne particles are present less radiation reaches the Earth's surface. Unfortunately, these measurements don’t work on cloudy days. AOD is converted to PM2.5 concentrations with statistical methods based on calibration and correction with FEM/FRM monitors. The authors reiterate that they think satellite data can do better than sensors to fill data gaps. They also note that satellite data can be used to determine the boundaries of non-attainment areas. States currently use five types of data to determine these boundaries: jurisdictional boundaries, air quality data, emissions data, geography and topography information, and weather data. They also use pollution modeling. EPA must approve non-attainment boundaries. The authors note: “Because pollution disperses, nonattainment boundaries work best when they err on the side of being more geographically expansive, rather than precisely drawn. High-resolution satellite data could provide for more tightly drawn boundary estimates, which may cut abatement costs in the long run, but erring on the side of public health with larger area boundaries seems wise, in general.”


    




     NASA also uses its ozone monitoring instrument (OMI) (launched in 2004) or TROPOspheric Monitoring Instrument (TROPOMI) (launched in 2017) satellites to measure tropospheric ozone but can also detect other pollutants and trace gases such as nitrogen dioxide, sulfur dioxide, and formaldehyde. These can track changes in NO2 pollution over time. They have been used to track increases in NO2 over active oil and gas basins such as the Williston Basin in Noth Dakota and the Permian Basin in West Texas and Southeast New Mexico. OMI trends of NO2 correlate well with surface measurements so its potential use for supplementing NO2 data is likely to be very good.

     Satellites can offer great geographical coverage, although accuracy and calibration can be considerably less reliable and both spatial and temporal resolution can be lower. In spite of these shortcomings, satellite data is well situated to track the movement of pollution plumes through the atmosphere.

    NASA has a brand new satellite up with the first test scans just released. This is the Tropospheric Emissions: Monitoring of Pollution instrument, or TEMPO. It takes hourly scans of North America, tracking air pollutant levels down to the neighborhood. It is expected to get an accurate estimate of rush-hour traffic pollution in major cities. The satellite was launched in April. The preliminary scans are from July 31 through August 2. It measures nitrogen oxides and other gases. 50 research studies are planned with the data once the satellite is up to full operation in October. The preliminary scans clearly show the elevated concentrations of NOx over cities, particularly Los Angeles.



Source: NASA




Source: NASA



 

Potential Use of Moss and Lichen to Detect and Quantify Heavy Metal Pollutants

 

     Sienna Bishop also notes some interesting studies done in the Pacific Northwest with moss and lichen to measure levels of toxic heavy metals such as cadmium and arsenic. Sampling is inexpensive and can cover a tight grid of local areas around known point sources to supplement other data and catch missed emission events.

 

 

Measurement Strategies for Methane Emissions from Oil & Gas Sites, Landfills, Sewage Treatment Facilities, Etc.

 

     Due to the desire to abate greenhouse gas emissions a whole industry has developed around methane emissions abatement, particularly around oil and gas sites. Though not a pollutant in the traditional sense, methane has a high global warming potential in the short-term (10-20 years) and contributes significantly to global heating. The industry also seeks to keep its ‘social license to operate’ by addressing these concerns. In order to do so, each site requires monitoring of methane emissions. In many cases involving emissions from certain equipment, methane emissions measurements are coupled with measurements of air pollutants like VOCs, so traditional air quality monitoring can be a co-benefit to methane emissions monitoring.

     The chief concern with methane emissions is methane escaping into the atmosphere, while the main concern with traditional pollutants is their concentration near the ground where humans live. Thus, the strategies for monitoring and abatement are a bit different. Methane is not considered to be toxic, but it is flammable and so is an explosion and fire hazard at higher levels.

     Equipment and protocols specific for measuring methane emissions include infrared optical imaging, stationary sensors, LiDAR that may be carried by drones, and satellite-based monitoring. Protocols have been developed to measure, verify, report, and certify emissions per facility and per company so that natural gas and oil sold by that company can be certified as methane abated.

 

References:

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US EPA, July 13, 2020. EPA and Wisconsin Announce All of Sheboygan County Now Meets Federal Air Quality Standard for Ozone. https://www.epa.gov/newsreleases/epa-and-wisconsin-announce-all-sheboygan-county-now-meets-federal-air-quality-standard

 

What Does the Air Recirculation Button in Your Car Actually Do? Sean Cate. August 14, 2023. The Premier Dailey. What Does the Air Recirculation Button in Your Car Actually Do? (msn.com)

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NASA now has an instrument orbiting Earth that can see major air pollutants across North America, tracing them down to an exact neighborhood. Katie Hawkinson. Business Insider. August 26, 2023. NASA now has an instrument orbiting Earth that can see major air pollutants across North America, tracing them down to an exact neighborhood (msn.com)

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